New technique shows promise for dramatic miniaturization of metamaterials and negative index of refraction of -700, one hundred times larger than before

In a vacuum, light travels so fast that it would circle the Earth more than seven times within the blink of an eye. When light propagates through matter, however, it slows by a factor typically less than 5. This factor, called the refractive index, is positive in naturally occurring materials, and it causes light to bend in a particular direction when it shines on, for example, water or glass.

Researchers at the Harvard School of Engineering and Applied Sciences (SEAS), collaborating with the Weizmann Institute of Science in Israel, have now demonstrated a drastically new way of achieving negative refraction in a metamaterial.

The advance, reported in the August 2 issue of Nature, results in an “extraordinarily strong” negative refractive index as large as -700, more than a hundred times larger than most previously reported.

“This work may bring the science and technology of negative refraction into an astoundingly miniaturized scale, confining the negatively refracting light into an area that is 10,000 times smaller than many previous negative-index metamaterials,” says principal investigator Donhee Ham, Gordon McKay Professor of Electrical Engineering and Applied Physics at SEAS.

a, Optical image of a 2DEG strip-array metamaterial prototype. Ground–signal–ground (GSG) on-chip CPWs direct electromagnetic waves to and from the metamaterial. The inset shows a magnified portion of the strip array.

Nature – A Newtonian approach to extraordinarily strong negative refraction

Over the past two decades, scientists have managed to create artificial materials whose refractive indices are negative; these negative-index metamaterials defy normal experience by bending light in the “wrong” direction. Due to their unusual ability to manipulate electromagnetic waves and their potential to be harnessed for technology (that might, for example, cloak objects from view), negative-index metamaterials have been celebrated by scientists and engineers alike.

The underlying physics of previous work in this field has often involved an entity called magnetic inductance. Ham’s research group instead explored kinetic inductance, which is the manifestation of the acceleration of electrons subjected to electric fields, according to Newton’s second law of motion.

At its heart, the researchers’ change in strategy from using magnetic inductance to kinetic inductance stems from a simple shift in ideas.

“Magnetic inductance represents the tendency of the electromagnetic world to resist change according to Faraday’s law,” explains Ham. “Kinetic inductance, on the other hand, represents the reluctance to change in the mechanical world, according to Newton’s law.”

“When electrons are confined perfectly into two dimensions, kinetic inductance becomes much larger than magnetic inductance, and it is this very large two-dimensional kinetic inductance that is responsible for the very strong negative refraction we achieve,” explains lead author Hosang Yoon, a graduate student at SEAS. “The dimensionality profoundly affects the condensed-matter electron behaviors, and one of those is the kinetic inductance.”

To obtain the large kinetic inductance, Ham and Yoon’s work employs a two-dimensional electron gas (2DEG), which forms at the interface of two semiconductors, gallium arsenide and aluminum gallium arsenide. The very “clean” 2DEG sample used in this work was fabricated by coauthor Vladimir Umansky, of the Weizmann Institute.

Ham’s team effectively sliced a sheet of 2DEG into an array of strips and used gigahertz-frequency electromagnetic waves (microwaves) to accelerate electrons in the leftmost few strips. The resulting movements of electrons in these strips were “felt” by the neighboring strips to the right, where electrons are consequently accelerated.

In this way, the proof-of-concept device propagates an effective wave to the right, in a direction perpendicular to the strips, each of which acts as a kinetic inductor due to the electrons’ acceleration therein. This effective wave proved to exhibit what the researchers call a “staggering” degree of negative refraction.

The primary advantages of the new technology are its ability to localize electromagnetic waves into ultra-subwavelength scales and its dramatically reduced size. This concept demonstrated with microwaves, if extended to other regions of the electromagnetic spectrum, may prove important for operating terahertz and photonic circuits far below their usual diffraction limit, and at near field. It may also one day lead to extremely powerful microscopes and optical tweezers, which are used to trap and study minuscule particles like viruses and individual molecules.

For now, the device operates at temperatures below 20 degrees Kelvin. The researchers note, however, that a similar result can be achieved at room temperature using terahertz waves, which Ham’s team is already investigating, with the carbon structure graphene as an alternative two-dimensional conductor.

“While electrons in graphene behave like massless particles, they still possess kinetic energy and can exhibit very large kinetic inductance in a non-Newtonian way,” says Ham.

The chamber of the probe station where Donhee Ham’s research group tests the new metamaterials. (Photo by Eliza Grinnell, SEAS Communications.)

ABSTRACT – Metamaterials with negative refractive indices can manipulate electromagnetic waves in unusual ways, and can be used to achieve, for example, sub-diffraction-limit focusing, the bending of light in the ‘wrong’ direction, and reversed Doppler and Cerenkov effects. These counterintuitive and technologically useful behaviours have spurred considerable efforts to synthesize a broad array of negative-index metamaterials with engineered electric, magnetic or optical properties. Here we demonstrate another route to negative refraction by exploiting the inertia of electrons in semiconductor two-dimensional electron gases, collectively accelerated by electromagnetic waves according to Newton’s second law of motion, where this acceleration effect manifests as kinetic inductance. Using kinetic inductance to attain negative refraction was theoretically proposed for three-dimensional metallic nanoparticles and seen experimentally with surface plasmons on the surface of a three-dimensional metal. The two-dimensional electron gas that we use at cryogenic temperatures has a larger kinetic inductance than three-dimensional metals, leading to extraordinarily strong negative refraction at gigahertz frequencies, with an index as large as −700. This pronounced negative refractive index and the corresponding reduction in the effective wavelength opens a path to miniaturization in the science and technology of negative refraction.

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